Ultrafast imaging of the Renner-Teller effect in a field-dressed molecule

Amini, K.; Steinle, T.; Sclafani, M.; Shaikh, M.; Sanchez, A.; Liu, X.; Le, A. T.; Steinmetzer, J.; Pfeifer, T.; Moshammer, R.; Ullrich, J.; Lewenstein, M.; Moszynski, R.; de Abajo, J. G.; Lin, C. D.; Graefe, S.; Biegert, J.

doi:10.1088/1742-6596/1412/9/092001

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Ultrafast imaging of the Renner-Teller effect in a field-dressed molecule

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Pfeifer, T.
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Moshammer, R.
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Citation

Amini, K., Steinle, T., Sclafani, M., Shaikh, M., Sanchez, A., Liu, X., et al. (2020). Ultrafast imaging of the Renner-Teller effect in a field-dressed molecule. Journal of Physics: Conference Series, 1412: 092001. doi:10.1088/1742-6596/1412/9/092001.

Cite as: https://hdl.handle.net/21.11116/0000-0008-19BA-B

Abstract

We present experimental results of linear-to-bent transition of field-dressed molecules, mediated by Renner-Teller effect. Using the state-of-the-art laser-induced electron diffraction (LIED) technique, we image a bent and symmetrically stretched carbon disulfide (CS2) molecule populating an excited electronic state under the influence of strong laser field. Our findings are well-supported by ab initio quantum mechanical calculations.