Large third‐order optical nonlinearity of the organic metal 
α‐[bis(ethylenedithio) tetrathiofulvalene] triiodide

Huggard, P. G.; Blau, W.; Schweitzer, D.

doi:10.1063/1.98933

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Large third‐order optical nonlinearity of the organic metal α‐[bis(ethylenedithio) tetrathiofulvalene] triiodide

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Schweitzer, D.
Department of Molecular Physics, Max Planck Institute for Medical Research, Max Planck Society;

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Citation

Huggard, P. G., Blau, W., & Schweitzer, D. (1987). Large third‐order optical nonlinearity of the organic metal α‐[bis(ethylenedithio) tetrathiofulvalene] triiodide. Applied Physics Letters, 51(26), 2183-2185. doi:10.1063/1.98933.

Cite as: https://hdl.handle.net/21.11116/0000-0008-2255-2

Abstract

The organic metal α‐[bis(ethylenedithio) tetrathiofulvalene]2I3 shows a large third‐order optical nonlinearity around 650 nm, as observed by forward degenerate four‐wave mixing. Nonlinear susceptibilities of ‖χ(3)‖ ∼5×10−8 esu are observed along the direction of maximum conductivity. The frequency dispersion of the nonlinearity points to a plasma effect due to the conduction electrons.