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In Situ Observation of Single-Molecule Surface Reactions from Low to High Affinities

MPS-Authors

Kim,  Eugene
Vollmer Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;
International Max Planck Research School, Max Planck Institute for the Science of Light, Max Planck Society;

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Baaske,  Martin D.
Vollmer Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

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Vollmer,  Frank
Vollmer Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

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Citation

Kim, E., Baaske, M. D., & Vollmer, F. (2016). In Situ Observation of Single-Molecule Surface Reactions from Low to High Affinities. Advanced Materials, 28(45), 9941-9948. doi:10.1002/adma.201603153.


Cite as: http://hdl.handle.net/21.11116/0000-0008-4D22-C
Abstract
In situ observation of single-molecule surface reactions from low to high affinities is achieved by resonant coupling between optical whispering-gallery modes and the localized surface plasmon of nanorods. Transient and permanent interactions between ligands (thiol, amine) and the gold surface are monitored without labels, allowing direct determination of the associated kinetic constants and rapid development of new functionalization protocols.