Delay-Induced Chaos in Catalytic Surface Reactions: NO Reduction on Pt(100)

Khrustova, N.; Veser, Götz; Mikhailov, Alexander S.; Imbihl, R.

doi:10.1103/PhysRevLett.75.3564

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Delay-Induced Chaos in Catalytic Surface Reactions: NO Reduction on Pt(100)

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Khrustova, N.
Fritz Haber Institute, Max Planck Society;

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Veser, Götz
Fritz Haber Institute, Max Planck Society;

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Mikhailov, Alexander S.
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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PhysRevLett.75.3564.pdf
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引用

Khrustova, N., Veser, G., Mikhailov, A. S., & Imbihl, R. (1995). Delay-Induced Chaos in Catalytic Surface Reactions: NO Reduction on Pt(100). Physical Review Letters, 75(19), 3564-3567. doi:10.1103/PhysRevLett.75.3564.

引用: https://hdl.handle.net/21.11116/0000-0008-CB73-2

要旨

Deterministic chaos has been observed in the NO+CO and NO+H₂ reactions on Pt(100). A mathematical model is proposed that explains the origin as being due to delays in the response of a population of reacting adsorbate islands globally coupled via the gas phase. The dynamical equations of this model yield a sequence of period-doubling bifurcations resulting in chaos.