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Fullerene-based ruthenium catalysts: a novel approach for anchoring metal to carbonaceous supports. I. Structure

MPS-Authors
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Braun,  Thomas
Fritz Haber Institute, Max Planck Society;

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Wohlers,  Michael
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Belz,  Thilo
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Uchida,  Yuji
Fritz Haber Institute, Max Planck Society;

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Pfänder,  Norbert
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Schlögl,  Robert
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Citation

Braun, T., Wohlers, M., Belz, T., Nowitzke, G., Wortmann, G., Uchida, Y., et al. (1997). Fullerene-based ruthenium catalysts: a novel approach for anchoring metal to carbonaceous supports. I. Structure. Catalysis Letters, 43(3-4), 167-173. doi:10.1023/A:1018998808208.


Cite as: https://hdl.handle.net/21.11116/0000-0008-E28D-A
Abstract
The influence of fullerenes and related support materials on the structural and catalytic properties of ruthenium was investigated. Catalysts based on C60, raw fullerene black, extracted fullerene black, cathode deposit and graphite were prepared by an impregnation/activation procedure with Ru3CO12. The local co-ordination sphere of the resulting highly dispersed X-ray amorphous ruthenium was investigated by means of EXAFS. The dominating role of the presence of non-six-membered carbon rings on the structure and the stability of the Ru particles will be illustrated