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Calculated lifetimes of hot electrons in aluminum and copper using a plane-wave basis set

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Schöne,  Wolf-Dieter
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Keyling,  Robert
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Bandic,  Mario
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Ekardt,  Walter
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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PhysRevB.60.8616.pdf
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Citation

Schöne, W.-D., Keyling, R., Bandic, M., & Ekardt, W. (1999). Calculated lifetimes of hot electrons in aluminum and copper using a plane-wave basis set. Physical Review B, 60(12), 8616-8623. doi:10.1103/PhysRevB.60.8616.


Cite as: https://hdl.handle.net/21.11116/0000-0008-F257-5
Abstract
We report about the lifetimes of hot electrons in crystalline aluminum and copper. For aluminum the results agree quantitatively with the experimental results. For copper we get good agreement for quasiparticle energies in the (110) direction above 2 eV which shows that the lifetimes for quasiparticle states above 2 eV are determined by sp bands, explaining the puzzling fact that simple Fermi liquid theory describes Cu in this direction quite well. The calculations were performed within the shielded interaction approximation using a plane-wave basis expansion for the wave functions. We show that for Cu this basis leads to equally good results as the more demanding linearized augmented plane-wave basis.