English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT

Released

Journal Article

Nature and impact of charge transfer to ground-state dications in atomic and molecular environments

MPS-Authors
/persons/resource/persons81302

Richter,  Clemens
Leibniz-Institut für Oberflächenmodifizierung (IOM);
Molecular Physics, Fritz Haber Institute, Max Planck Society;

/persons/resource/persons109362

Hergenhahn,  Uwe
Leibniz-Institut für Oberflächenmodifizierung (IOM);
Molecular Physics, Fritz Haber Institute, Max Planck Society;

External Resource
No external resources are shared
Fulltext (restricted access)
There are currently no full texts shared for your IP range.
Fulltext (public)

PhysRevA.104.042802.pdf
(Publisher version), 593KB

Supplementary Material (public)
There is no public supplementary material available
Citation

Küstner-Wetekam, C., Hu, X. Q., Marder, L., Schmidt, P., Ozga, C., Zindel, C., et al. (2021). Nature and impact of charge transfer to ground-state dications in atomic and molecular environments. Physical Review A, 104(4): 042802. doi:10.1103/PhysRevA.104.042802.


Cite as: https://hdl.handle.net/21.11116/0000-0009-65A0-0
Abstract
Charge transfer processes between weakly bound entities play an important role in various chemical and biological environments. In this combined experimental and theoretical work, we investigate the nature of charge-transfer processes in homogeneous atomic and heterogeneous atomic-molecular clusters. Our results reveal fundamentally different processes to be at play in pure argon clusters compared to mixed argon-nitrogen systems: We demonstrate that the former species decay via photon-mediated charge transfer while a nonradiative direct process is found dominant in the atomic-molecular cases. Our results are of general interest for studies on charge redistribution in more complex and biologically relevant samples where molecules are involved.