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Journal Article

Photoelectron Soft X-Ray Fluorescence Coincidence Spectroscopy on Free Molecules

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Neeb,  M.
Fritz Haber Institute, Max Planck Society;

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PhysRevLett.76.3919.pdf
(Publisher version), 73KB

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Citation

Rubensson, J.-E., Lüning, J., Neeb, M., Küpper, B., Eisebitt, S., & Eberhardt, W. (1996). Photoelectron Soft X-Ray Fluorescence Coincidence Spectroscopy on Free Molecules. Physical Review Letters, 76(21), 3919-3922. doi:10.1103/PhysRevLett.76.3919.


Cite as: https://hdl.handle.net/21.11116/0000-0009-AB1C-8
Abstract
A technique for measuring core-level photoemission from free molecules in coincidence with the soft x-ray fluorescence decay is presented. Zero-kinetic-energy photoelectrons are detected in a time-of-flight electron spectrometer, and photons are collected in a large solid angle by a detector situated close to the interaction region. The coincidence spectrum of N2 shows an adiabatic 1s line, free from electron-electron postcollision interaction effects. The results open up new aspects on core-hole excitation-emission dynamics.