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Time-Resolved Two-Color Photoelectron Spectroscopy at Bare and Adsorbate Covered Metal Surfaces

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Hertel,  Tobias
Physical Chemistry, Fritz Haber Institute, Max Planck Society;
IBM Research Division;

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Knoesel,  Ernst
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Wolf,  Martin
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Ertl,  Gerhard
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Citation

Hertel, T., Knoesel, E., Wolf, M., & Ertl, G. (1996). Time-Resolved Two-Color Photoelectron Spectroscopy at Bare and Adsorbate Covered Metal Surfaces. In P. F. Barbara, J. G. Fujimoto, W. H. Knox, & W. Zinth (Eds.), Ultrafast Phenomena X (1, pp. 448-449). Berlin, Heidelberg: Springer.


Cite as: https://hdl.handle.net/21.11116/0000-0009-B020-B
Abstract
We investigate the influence of rare-gas (Xe, Kr) overlayers on the ultra-fast dynamics of photoexcited electrons in image-potential states on Cu(111). A density matrix calculation using the Liouville-von-Neumann equation gives a fully consistent description of the time-dependent two-photon photoemission process. Our studies provide new insights into electronic dephasing at metal surfaces.