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Journal Article

Photoelectron circular dichroism in angle-resolved photoemission from liquid fenchone

MPS-Authors
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Pohl,  Marvin Nicolas
Molecular Physics, Fritz Haber Institute, Max Planck Society;
Department of Chemistry, University of California;
Chemical Sciences Division, Lawrence Berkeley National Laboratory;

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Malerz,  Sebastian
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Trinter,  Florian
Molecular Physics, Fritz Haber Institute, Max Planck Society;
Institut für Kernphysik, Goethe-Universität Franfurt am Main;

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Kolbeck,  Claudia
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Meijer,  Gerard
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Winter,  Bernd
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Hergenhahn,  Uwe       
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Citation

Pohl, M. N., Malerz, S., Trinter, F., Lee, C., Kolbeck, C., Wilkinson, I., et al. (2022). Photoelectron circular dichroism in angle-resolved photoemission from liquid fenchone. Physical Chemistry Chemical Physics, 24(14), 8081-8092. doi:10.1039/d1cp05748k.


Cite as: https://hdl.handle.net/21.11116/0000-000A-256B-5
Abstract
We present an experimental X-ray photoelectron circular dichroism (PECD) study of liquid fenchone at the C 1s edge. A novel setup to enable PECD measurements on a liquid microjet [Malerz et al., Rev. Sci. Instrum., 2022, 93, 015101] was used. For the C 1s line assigned to fenchone's carbonyl carbon, a non-vanishing asymmetry is found in the intensity of photoelectron spectra acquired under a fixed angle in the backward-scattering plane. This experiment paves the way towards an innovative probe of the chirality of organic/biological molecules in aqueous solution.