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Long-wave infrared super-resolution wide-field microscopy using sum-frequency generation

MPS-Authors
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Niemann,  Richarda
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Waßerroth,  Sören
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Gewinner,  Sandy
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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De Pas,  Marco
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Schöllkopf,  Wieland
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Wolf,  Martin
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Paarmann,  Alexander
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Citation

Niemann, R., Waßerroth, S., Lu, G., Gewinner, S., De Pas, M., Schöllkopf, W., et al. (2022). Long-wave infrared super-resolution wide-field microscopy using sum-frequency generation. Applied Physics Letters, 120(13): 131102. doi:10.1063/5.0081817.


Cite as: https://hdl.handle.net/21.11116/0000-000A-32F0-E
Abstract
Super-resolution microscopy in the visible is an established powerful tool in various disciplines. In the long-wave infrared (LWIR) spectral range, however, no comparable schemes have been demonstrated to date. In this work, we experimentally demonstrate super-resolution microscopy in the LWIR range (λIR ≈ 10–12 μm) using IR-visible sum-frequency generation. We operate our microscope in a wide-field scheme and image localized surface phonon polaritons in 4H-SiC nanostructures as a proof-of-concept. With this technique, we demonstrate an enhanced spatial resolution of ~λIR/9, enabling to resolve the polariton resonances in individual sub-diffractional nanostructures with sub-wavelength spacing. Furthermore, we show that this resolution allows us to differentiate between spatial patterns associated with different polariton modes within individual nanostructures.