English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse
  1. View item / 
  2. Item Summary

Item

ITEM ACTIONSEXPORT
Add to Basket
  Local TagsRelease HistoryDetailsSummary

Released
Journal Article

Experimental and Theoretical Advances on Single Atom and Atomic Cluster-Decorated Low-Dimensional Platforms towards Superior Electrocatalysts

MPS-Authors
/persons/resource/persons267642

He,  Tianwei
Theory, Fritz Haber Institute, Max Planck Society;

External Resource
No external resources are shared
Fulltext (restricted access)
There are currently no full texts shared for your IP range.
Fulltext (public)
Supplementary Material (public)
There is no public supplementary material available
Citation

He, T., Puente-Santiago, A. R., Xia, S., Ahsan, M. A., Xu, G., & Luque, R. (2022). Experimental and Theoretical Advances on Single Atom and Atomic Cluster-Decorated Low-Dimensional Platforms towards Superior Electrocatalysts. Advanced Energy Materials, 12(22): 2200493. doi:10.1002/aenm.202200493.


Cite as: https://hdl.handle.net/21.11116/0000-000A-76B6-4
Abstract
The fundamental relationship between structure and properties, which is called “structure-property”, plays a vital role in the rational designing of high-performance catalysts for diverse electrocatalytic applications. Low-dimensional (LD) nanomaterials, including 0D, 1D, 2D materials, combined with low-nuclearity metal atoms, ranging from single atoms to subnanometer clusters, are currently emerging as rising star nanoarchitectures for heterogeneous catalysis due to their well-defined active sites and unbeatable metal utilization efficiencies. In this work, a comprehensive experimental and theoretical review is provided on the recent development of single atom and atomic cluster-decorated LD platforms towards some typical clean energy reactions, such as water-splitting, nitrogen fixation, and carbon dioxide reduction reactions. The upmost attractive structural properties, advanced characterization techniques, and theoretical principles of these low-nuclearity electrocatalysts as well as their applications in key electrochemical energy devices are also elegantly discussed.