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Journal Article

Extreme Ultraviolet Wave Packet Interferometry of the Autoionizing HeNe Dimer

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Trinter,  Florian
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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acs.jpclett.2c01619.pdf
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Citation

Uhl, D., Wituschek, A., Michiels, R., Trinter, F., Jahnke, T., Allaria, E., et al. (2022). Extreme Ultraviolet Wave Packet Interferometry of the Autoionizing HeNe Dimer. The Journal of Physical Chemistry Letters, 13(36), 8470-8476. doi:10.1021/acs.jpclett.2c01619.


Cite as: https://hdl.handle.net/21.11116/0000-000B-16EE-1
Abstract
Femtosecond extreme ultraviolet wave packet interferometry (XUV-WPI) was applied to study resonant interatomic Coulombic decay (ICD) in the HeNe dimer. The high demands on phase stability and sensitivity for vibronic XUV-WPI of molecular-beam targets are met using an XUV phase-cycling scheme. The detected quantum interferences exhibit vibronic dephasing and rephasing signatures along with an ultrafast decoherence assigned to the ICD process. A Fourier analysis reveals the molecular absorption spectrum with high resolution. The demonstrated experiment shows a promising route for the real-time analysis of ultrafast ICD processes with both high temporal and high spectral resolution.