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Journal Article

Three-dimensional Fermi surfaces from charge order in layered CsV3Sb5

MPS-Authors
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Guo,  C.
Laboratory of Quantum Materials (QMAT), Institute of Materials (IMX), École Polytechnique Fédérale de Lausanne (EPFL);
Microstructured Quantum Matter Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

/persons/resource/persons242811

Putzke,  C.
Laboratory of Quantum Materials (QMAT), Institute of Materials (IMX), École Polytechnique Fédérale de Lausanne (EPFL);
Microstructured Quantum Matter Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

/persons/resource/persons191608

Moll,  P. J. W.
Laboratory of Quantum Materials (QMAT), Institute of Materials (IMX), École Polytechnique Fédérale de Lausanne (EPFL);
Microstructured Quantum Matter Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

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PhysRevB.106.064510.pdf
(Publisher version), 2MB

Supplementary Material (public)

Cs135_SI.pdf
(Supplementary material), 110KB

Citation

Huang, X., Guo, C., Putzke, C., Gutierrez-Amigo, M., Sun, Y., Vergniory, M. G., et al. (2022). Three-dimensional Fermi surfaces from charge order in layered CsV3Sb5. Physical Review B, 106(6): 064510. doi:10.1103/PhysRevB.106.064510.


Cite as: https://hdl.handle.net/21.11116/0000-000B-337D-0
Abstract
The cascade of electronic phases in CsV3Sb5 raises the prospect to disentangle their mutual interactions in a clean, strongly interacting kagome lattice. When the kagome planes are stacked into a crystal, its electronic dimensionality encodes how much of the kagome physics and its topological aspects survive. The layered structure of CsV3Sb5 reflects in Brillouin-zone-sized quasi-two-dimensional Fermi surfaces and significant transport anisotropy. Yet here we demonstrate that CsV3Sb5 is a three-dimensional (3D) metal within the charge density wave (CDW) state. Small 3D pockets play a crucial role in its low-temperature magneto- and quantum transport. Their emergence at TCDW≈93K results in an anomalous sudden increase of the in-plane magnetoresistance by four orders of magnitude. The presence of these 3D pockets is further confirmed by quantum oscillations under in-plane magnetic fields, demonstrating their closed nature. These results emphasize the impact of interlayer coupling on the kagome physics in 3D materials.