Triplet excitations of crystalline C60. An optically detected 
magnetic-resonance study in zero field

Matsushita, M.; Frens, A.M.; Groenen, E.J.J.; Poluektov, O.G.; Schmidt, J.; Meijer, Gerard; Verheijen, M.A.

doi:10.1016/0009-2614(93)85648-8

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Triplet excitations of crystalline C₆₀. An optically detected magnetic-resonance study in zero field

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Matsushita, M., Frens, A., Groenen, E., Poluektov, O., Schmidt, J., Meijer, G., et al. (1993). Triplet excitations of crystalline C₆₀. An optically detected magnetic-resonance study in zero field. Chemical Physics Letters, 214(3-4), 349-352. doi:10.1016/0009-2614(93)85648-8.

Cite as: https://hdl.handle.net/21.11116/0000-000C-157B-3

Abstract

Upon excitation of a single crystal of C₆₀ in the visible, microwave transitions have been detected optically in zero field. The transitions derive from triplet states and their frequencies verify that these states are delocalized over more than one C₆₀ molecule, as previously inferred from EPR experiments. Different triplet states seem to correspond to excitations that are trapped in different domains of the crystal which indicates that structural or impurity-induced defects may be involved.