High-resolution study of the NO E 2Σ+ ← A 2Σ+ transition by pulsed-cw double 
resonance

Meijer, Gerard; Ebben, Maarten; Meulen, J.J. ter

doi:10.1016/0009-2614(88)80261-6

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High-resolution study of the NO E ²Σ⁺ ← A ²Σ⁺ transition by pulsed-cw double resonance

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Citation

Meijer, G., Ebben, M., & Meulen, J. t. (1988). High-resolution study of the NO E ²Σ⁺ ← A ²Σ⁺ transition by pulsed-cw double resonance. Chemical Physics Letters, 147(6), 525-528. doi:10.1016/0009-2614(88)80261-6.

Cite as: https://hdl.handle.net/21.11116/0000-000C-3C42-7

Abstract

A new experimental technique which combines the high power of a pulsed laser with the narrow bandwidth of a single mode cw laser has been used to study the NO (E ²Σ⁺, ν = 0 ← A ²Σ⁺, ν = 0) transition under high resolution in a molecular beam. The spin-rotation splitting in the E state has been analyzed and shows the effect of a heterogeneous perturbation between the E ²Σ⁺, ν = 0 and the B ²Π, ν = 17 state. Time-resolved E→A fluorescence spectra show redisual effects of Rabi oscillations and can be correctly described using the optical Bloch equations for a two-level system, including radiative losses.