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Journal Article

On-chip interference of scattering from two individual molecules

MPS-Authors
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Rattenbacher,  Dominik
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

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Shkarin,  Alexey
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Renger,  Jan
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Utikal,  Tobias
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Götzinger,  Stephan
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

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Sandoghdar,  Vahid
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;
Sandoghdar Division, Max-Planck-Zentrum für Physik und Medizin, Max Planck Institute for the Science of Light, Max Planck Society;

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Citation

Rattenbacher, D., Shkarin, A., Renger, J., Utikal, T., Götzinger, S., & Sandoghdar, V. (2023). On-chip interference of scattering from two individual molecules. Optica, 10, 1595-1601. doi:10.1364/OPTICA.502221.


Cite as: https://hdl.handle.net/21.11116/0000-000C-7CE4-8
Abstract
Integrated photonic circuits offer a promising route for studying coherent cooperative effects of a controlled collection of quantum emitters. However, spectral inhomogeneities, decoherence, and material incompatibilities in the solid state make this a nontrivial task. Here, we demonstrate efficient coupling of a pair of Fourier-limited organic molecules embedded in a polyethylene film to a TiO2 microdisc resonator on a glass chip. Moreover, we tune the resonance frequencies of the emitters with respect to that of the microresonator by employing nanofabricated electrodes. For two molecules separated by a distance of about 8 µm and an optical phase difference of about pi/2, we report on a large collective extinction of the incident light in the forward direction and the destructive interference of its scattering in the backward direction. Our work sets the ground for coherent coupling of several quantum emitters via a common mode and realization of polymer-based hybrid quantum photonic circuits.