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Journal Article

Ligand-to-Copper Charge-Transfer-Enabled C–H Sulfoximination of Arenes

MPS-Authors
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Su,  Wanqi
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;
Institute of Organic Chemistry, RWTH Aachen University;

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Xu,  Peng
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Petzold,  Roland
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Yan,  Jiyao
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;
Institute of Organic Chemistry, RWTH Aachen University;

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Ritter,  Tobias
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Citation

Su, W., Xu, P., Petzold, R., Yan, J., & Ritter, T. (2023). Ligand-to-Copper Charge-Transfer-Enabled C–H Sulfoximination of Arenes. Organic Letters, 25(6), 1025-1029. doi:10.1021/acs.orglett.3c00256.


Cite as: https://hdl.handle.net/21.11116/0000-000C-BA5F-9
Abstract
Herein, we report a photoinduced sulfoximine-to-copper charge-transfer-enabled generation of sulfoximinyl radicals directly from NH-sulfoximines for C–H sulfoximination of arenes via radical addition. Through copper-LMCT, N-arylation of NH-sulfoximines was achieved for the first time using arenes of different electronic structures as the aryl donors.