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Spectral splitting of a stimulated Raman transition in a single molecule

MPG-Autoren
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Zirkelbach,  Johannes
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

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Gürlek,  Burak
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

/persons/resource/persons270607

Mirzaei,  Masoud
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

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Shkarin,  Alexey
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

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Utikal,  Tobias
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

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Götzinger,  Stephan
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;

/persons/resource/persons201175

Sandoghdar,  Vahid
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;
Friedrich-Alexander-Universität Erlangen-Nürnberg, External Organizations;
Sandoghdar Division, Max-Planck-Zentrum für Physik und Medizin, Max Planck Institute for the Science of Light, Max Planck Society;

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PhysRevResearch.5.043244.pdf
(Verlagsversion), 2MB

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Zitation

Zirkelbach, J., Gürlek, B., Mirzaei, M., Shkarin, A., Utikal, T., Götzinger, S., et al. (2023). Spectral splitting of a stimulated Raman transition in a single molecule. Physical Review Research, 5: 043244. doi:10.1103/PhysRevResearch.5.043244.


Zitierlink: https://hdl.handle.net/21.11116/0000-000C-BAE5-0
Zusammenfassung
The small cross-section of Raman scattering poses a great challenge for its direct study at the single-molecule level. By exploiting the high Franck-Condon factor of a common-mode resonance, choosing a large vibrational frequency difference in electronic ground and excited states and operating at T<2K, we succeed at driving a coherent stimulated Raman transition in individual molecules. We observe and model a spectral splitting that serves as a characteristic signature of the phenomenon at hand. Our study sets the ground for exploiting the intrinsic optomechanical degrees of freedom of molecules for applications in solid-state quantum optics and information processing.