Photon pumping, photodissociation and dissipation at interplay for the 
fluorescence of a molecule in a cavity

Gopalakrishna, M.; Viñas Boström, E.; Verdozzi, C.

doi:10.21468/SciPostPhys.15.4.138

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Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity

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Viñas Boström, E.
Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

Externe Ressourcen

https://arxiv.org/abs/2302.08966
(Preprint)

https://doi.org/10.21468/SciPostPhys.15.4.138
(Verlagsversion)

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Zitation

Gopalakrishna, M., Viñas Boström, E., & Verdozzi, C. (2023). Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity. SciPost Physics, 15(4): 138. doi:10.21468/SciPostPhys.15.4.138.

Zitierlink: https://hdl.handle.net/21.11116/0000-000C-CD01-C

Zusammenfassung

We introduce a model description of a diatomic molecule in an optical cavity, with pump and fluorescent fields, and electron and nuclear motion are treated on equal footing and exactly. The model accounts for several optical response temporal scenarios: A Mollow spectrum hindered by electron correlations, a competition of harmonic generation and molecular dissociation, a dependence of fluorescence on photon pumping rate and dissipation. It is thus a general and flexible template for insight into experiments where quantum photon confinement, leakage, nuclear motion and electronic correlations are at interplay.