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Preprint

Hybrid THz architectures for molecular polaritonics

MPS-Authors

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Reitz, Michael
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

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Genes, Claudiu
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

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Citation

Jaber, A., Reitz, M., Singh, A., Maleki, A., Xin, Y., Sullivan, B., et al. (in preparation). Hybrid THz architectures for molecular polaritonics.

Abstract

We explore several schemes of electromagnetic field confinement aimed at
facilitating the collective strong coupling of a localized photonic mode to
molecular vibrations in the terahertz region. The key aspects are the use of
plasmonic metasurface structures combined with standard Fabry-Perot
configurations and the deposition of a thin layer of glucose, via a spray
coating technique, within a tightly focused electromagnetic mode volume. We
observe vacuum Rabi splittings reaching up to 140 GHz and study the complex
interplay between plasmonic resonances, photonic cavity modes and low-energy
molecular resonances. Our study provides key insight into the design of
polaritonic platforms with organic molecules to harvest the unique properties
of hybrid light-matter states.