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Mott versus Slater-type metal-insulator transition in Mn-substituted Sr3Ru2O7

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Bohnenbuck,  B.
Department Solid State Spectroscopy (Bernhard Keimer), Max Planck Institute for Solid State Research, Max Planck Society;

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Keimer,  B.
Department Solid State Spectroscopy (Bernhard Keimer), Max Planck Institute for Solid State Research, Max Planck Society;

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Sawatzky,  G. A.
External Scientific Members, Max Planck Institute for Solid State Research, Max Planck Society;
Miscellaneous, Max Planck Institute for Solid State Research, Max Planck Society;

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Damascelli,  A.
Department Solid State Spectroscopy (Bernhard Keimer), Max Planck Institute for Solid State Research, Max Planck Society;

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Citation

Hossain, M. A., Bohnenbuck, B., Chuang, Y. D., Haverkort, M. W., Elfimov, I. S., Tanaka, A., et al. (2012). Mott versus Slater-type metal-insulator transition in Mn-substituted Sr3Ru2O7. Physical Review B, 86(4): 041102(R).


Cite as: https://hdl.handle.net/21.11116/0000-000E-C355-6
Abstract
We present a temperature-dependent x-ray-absorption (XAS) and resonant elastic x-ray scattering (REXS) study of the metal-insulator transition (MIT) in Sr-3(Ru1-xMnx)(2)O-7. The XAS results reveal that the MIT drives the onset of local antiferromagnetic correlations around the Mn impurities, a precursor of the long-range antiferromagnetism detected by REXS at T-order < T-MIT. This establishes that the MIT is of the Mott type (electronic correlations) as opposed to Slater type (magnetic order). While this behavior is induced by Mn impurities, the (1/4, 1/4, 0) order exists for a wide range of Mn concentrations, and points to an inherent instability of Sr3Ru2O7.