English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT

Released

Journal Article

Mechanism of the Far-Infrared Absorption of Carbon-Nanotube Films

MPS-Authors
/persons/resource/persons21693

Kampfrath,  Tobias
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

/persons/resource/persons22203

von Volkmann,  Konrad
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

/persons/resource/persons21762

Krenz,  Marcel
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

/persons/resource/persons21531

Frischkorn,  Christian
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

/persons/resource/persons22250

Wolf,  Martin
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

External Resource
No external resources are shared
Fulltext (restricted access)
There are currently no full texts shared for your IP range.
Fulltext (public)

428743.pdf
(Any fulltext), 284KB

Supplementary Material (public)
There is no public supplementary material available
Citation

Kampfrath, T., von Volkmann, K., Aguirre, C. M., Desjardins, P., Martel, R., Krenz, M., et al. (2008). Mechanism of the Far-Infrared Absorption of Carbon-Nanotube Films. Physical Review Letters, 101(26): 267403. doi:10.1103/PhysRevLett.101.267403.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0010-FB43-7
Abstract
The far-infrared conductivity of single-wall carbon-nanotube ensembles is dominated by a broad absorption peak around 4THz whose origin is still debated. We observe an overall depletion of this peak when the nanotubes are excited by a short visible laser pulse. This finding excludes optical absorption due to a particle-plasmon resonance and instead shows that interband transitions in tubes with an energy gap of ~10 meV dominate the far-infrared conductivity. A simple model based on an ensemble of two-level systems naturally explains the weak temperature dependence of the far-infrared conductivity by the tube-to-tube variation of the chemical potential.