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Spectroscopic Fingerprints of Amine and Imide Functional Groups in Self-Assembled Monolayers

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Kampen,  Thorsten U.
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Schmidt-Weber,  Philipp Martin
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Horn,  Karsten
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Citation

Ruiz-Osés, M., Kampen, T. U., González-Lakunza, N., Silanes, I., Schmidt-Weber, P. M., Gourdon, A., et al. (2007). Spectroscopic Fingerprints of Amine and Imide Functional Groups in Self-Assembled Monolayers. ChemPhysChem, 8(11), 1722-1726. doi:10.1002/cphc.200700295.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0011-0067-1
Abstract
The electronic structures of naphthalene tetracarboxylic diimide (NTCDI) and 1,4-bis(4,6-diamino-1,3,5-triazin-2-yl)benzene (BDG) monolayer assemblies grown on Au(111) are investigated by photoemission spectroscopy, X-ray absorption, and density functional theory. The different spectroscopic features in the absorption and core-level photoemission spectra are understood in terms of contributions from different core and molecular levels at N- and O-atom sites. This study provides clear spectroscopic fingerprints for amine and imide functional end groups, which drive the self-organization process in a number of planar, π-conjugated molecular structures.X-ray absorption spectroscopy