Orientation of nitrous oxide on palladium(110) by STM

Watanabe, Kazuo; Kokalj, Anton; Inokuchi, Yoshiya; Rzeznicka, Izabela; Ohshimo, Keijiro; Nishi, Nobuyuki; Matsushima, Tatsuo

doi:10.1016/j.cplett.2005.03.033

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Orientation of nitrous oxide on palladium(110) by STM

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Watanabe, Kazuo
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Citation

Watanabe, K., Kokalj, A., Inokuchi, Y., Rzeznicka, I., Ohshimo, K., Nishi, N., et al. (2005). Orientation of nitrous oxide on palladium(110) by STM. Chemical Physics Letters, 406(4-6), 474-478. doi:10.1016/j.cplett.2005.03.033.

Cite as: https://hdl.handle.net/11858/00-001M-0000-0011-08BF-A

Abstract

The adsorption structure of N2O on Pd(1 1 0) was analyzed below 14 K by scanning-tunneling microscopy. The N2O monomer was oriented along the [0 0 1] direction in the on-top form. Furthermore, the formation of small aggregates extending along the [1-1 0] direction was observed. The observed images were well-simulated for two types of cluster structures optimized by density-functional theory calculations. The components in the aggregates are proposed to be in a tilted form either on bridge sites or on-top sites.