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Journal Article

Nearest-neighbor-atom core-hole transfer in isolated molecules

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Rolles,  Daniel
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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e223002.pdf
(Publisher version), 113KB

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Citation

Guillemin, R., Hemmers, O., Rolles, D., Yu, S., Wolska, A., Tran, I., et al. (2004). Nearest-neighbor-atom core-hole transfer in isolated molecules. Physical Review Letters, 92(22), 223002-1-223002-4. doi:10.1103/PhysRevLett.92.223002.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0011-0C5A-A
Abstract
A new phenomenon sensitive only to next-door-neighbor atoms in isolated molecules is demonstrated using angle-resolved photoemission of site-selective core electrons. Evidence for this interatomic core-to-core electron interaction is observable only by measuring nondipolar angular distributions of photoelectrons. In essence, the phenomenon acts as a very fine atomic-scale sensor of nearest-neighbor elemental identity.