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Laser temperature jump experiments with micrometre space resolution using Rhodamine 101 anti-Stokes fluorescence from nanoseconds to milliseconds

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Holzwarth,  Josef F.
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Couderc,  Sabine
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Citation

Holzwarth, J. F., Couderc, S., Beeby, A., Parker, A. W., & Clark, I. P. (2003). Laser temperature jump experiments with micrometre space resolution using Rhodamine 101 anti-Stokes fluorescence from nanoseconds to milliseconds. In B. Wyborn (Ed.), Central Laser Facility Annual Report 2002/2003 (pp. 131-132). Chilton, Didcot, Oxfordshire, OX11 0QX; UK: CCLRC Rutherford Appelton Laboratory.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0011-0F32-E
Abstract
The investigation of dynamic changes in solutions is very important in learning about reaction mechanisms. The laser temperature jump technique, which uses the solvent as energy absorber, allows the observation of kinetic events over a time scale from 100 ps to 1 s, and offers the possibility to produce temperature changes in volumes of a microlitre or less.