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Dissolved Carbon Controls the Initial Stages of Nanocarbon Growth

MPS-Authors
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Rinaldi,  Ali
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Tessonnier,  Jean-Philippe
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Schuster,  Manfred Erwin
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Blume,  Raoul
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Girgsdies,  Frank
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Zhang,  Qiang
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Su,  Dang Sheng
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;
Shenyang National Laboratory for Materials Science Institute of Metal Research, Chinese Academy of Science;

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Schlögl,  Robert
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Citation

Rinaldi, A., Tessonnier, J.-P., Schuster, M. E., Blume, R., Girgsdies, F., Zhang, Q., et al. (2011). Dissolved Carbon Controls the Initial Stages of Nanocarbon Growth. Angewandte Chemie International Edition, 50(14), 3313-3317. doi:10.1002/anie.201006639.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0011-5366-E
Abstract
Sneaked in: Carbon atoms from defective supports are incorporated in nickel nanoparticles at relatively low temperatures (for example in a Ni(100) surface; Ni brown, C black) The dissolved carbon not only modifies the electronic properties of the metal but it also leads to a reconstruction of the nanoparticles. These findings may explain many of the differences in catalytic activity observed when supporting metals on carbon.