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Breakup dynamics and the isotope effect in H3+ and D 3+ dissociative recombination

MPS-Authors
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Strasser,  D.
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Lammich,  L.
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Kreckel,  H.
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Krohn,  S.
Prof. Dirk Schwalm, Emeriti, MPI for Nuclear Physics, Max Planck Society;

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Lange,  M.
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Schwalm,  D.
Prof. Dirk Schwalm, Emeriti, MPI for Nuclear Physics, Max Planck Society;

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Wolf,  A.
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Zajfman,  D.
Prof. Dirk Schwalm, Emeriti, MPI for Nuclear Physics, Max Planck Society;

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Citation

Strasser, D., Lammich, L., Kreckel, H., Krohn, S., Lange, M., Naaman, A., et al. (2002). Breakup dynamics and the isotope effect in H3+ and D 3+ dissociative recombination. Physical Review A (Atomic, Molecular, and Optical Physics), 66, 032719 -1-032719 -13.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0011-84F3-B
Abstract
The breakup dynamics of H3+ and D3+ following dissociative recombination is studied using the combination of two-dimensional imaging and storage ring techniques. The vibrational distributions of the molecular H2 and D2 fragments produced in the two body fragmentation channel were measured, as well as the kinematical correlation between the hydrogen or deuterium atoms produced in the three body channel. For the latter, we find predominantly linear dissociation geometries. The data also show that the initial molecular ions H3+and D3+, which were stored and electron cooled for up to 40 s prior to recombination, are still rotationally hot.