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Fragmentation of molecules studied with laser-induced Coulomb explosion imaging and femtosecond pump-probe experiments

MPG-Autoren
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Ergler,  Th.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Rudenko,  A.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Feuerstein,  B.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Zrost,  K.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Schröter,  C.D.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Moshammer,  R.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Ullrich,  J.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Zitation

Ergler, T., Rudenko, A., Feuerstein, B., Zrost, K., Schröter, C., Moshammer, R., et al. (2006). Fragmentation of molecules studied with laser-induced Coulomb explosion imaging and femtosecond pump-probe experiments. Proceedings of SPIE, 62560C: 62560C.


Zitierlink: http://hdl.handle.net/11858/00-001M-0000-0011-86C9-E
Zusammenfassung
We report on the experimental realisation of time-resolved coincident Coulomb explosion imaging of H2-fragmentation in 1014 W/cm2 laser fields. Combining a high-resolution 'reaction microscope' and a fs pump-probe setup, we map the motion of wave packets dissociating via one- or two-photon channels, respectively, and observe two region of enhanced ionization in accordance with earlier theoretical predictions. The long-term interferometric stability of our system allows us to extend pump-probe experiments into the region of overlapping pulses, which offers new possibilities for the manipulation of ultrafast molecular fragmentation dynamics.