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Abstract

We present a novel spectroscopic method based on a phase-modulated interferometer which is suitable for the high-precision measurement of absorption and index of refraction profiles. A comparison with competing methods, that is with interferometry and mil spectroscopy, is given. The combination of these two methods, the phase-modulated interferometer, is shown to be best suited for experiments aiming at the realization of novel optical media, for example media exhibiting an ultra-large index of refraction or strong dispersion without absorption. The theory of operation and a theoretical and experimental signal-to-noise analysis are presented. Current detection limits for optical phase shift and relative absorption are 1.1 x 10(-5) rad/root Hz and 2x10(-5)/root Hz, respectively. We demonstrate the effectiveness of this novel technique by investigating the absorption and index of refraction profiles of the 4s(2) S-1(0) --> 4s4p P-1(1) resonance transition at 423 nm in calcium