Self-assembled carbon nitride for photocatalytic hydrogen evolution and 
degradation of p-nitrophenol

Sun, Jingwen; Xu, Jingsan; Grafmueller, Andrea; Huang, Xing; Liedel, Clemens; Algara-Siller, Gerardo; Willinger, Marc Georg; Yang, Can; Fu, Yongsheng; Wang, Xin; Shalom, Menny

doi:10.1016/j.apcatb.2016.12.030

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Self-assembled carbon nitride for photocatalytic hydrogen evolution and degradation of p-nitrophenol

MPS-Authors

Sun, Jingwen
Key Laboratory of Soft Chemistry and Functional Materials, Nanjing University of Science and Technology, Ministry of Education;
Marc Willinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

Xu, Jingsan
Marc Willinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;
Menny Shalom, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Huang, Xing
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

Liedel, Clemens
Clemens Liedel, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Algara-Siller, Gerardo
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

Willinger, Marc Georg
Marc Willinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

Shalom, Menny
Menny Shalom, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;
Chemistry Department, Ben Gurion University of the Negev;

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引用

Sun, J., Xu, J., Grafmueller, A., Huang, X., Liedel, C., Algara-Siller, G., Willinger, M. G., Yang, C., Fu, Y., Wang, X., & Shalom, M. (2017). Self-assembled carbon nitride for photocatalytic hydrogen evolution and degradation of p-nitrophenol. Applied Catalysis B, 205, 1-10. doi:10.1016/j.apcatb.2016.12.030.

引用: https://hdl.handle.net/11858/00-001M-0000-002C-4E18-F

要旨

Carbon nitride has attracted significant interest as robust, low-cost alternative to metal-based materials in fields such as photo, electro and heterogeneous catalysis. However, the properties of the final material are hard to control by traditional synthetic methods Herein, we introduce a new strategy of material design that allows controlling the desired properties of the final material already from the molecular level by sequential solvent treatment of supramolecular aggregates that serve as the reactants. Due to in situ formation of a thermodynamic driven energy levels gradient, the as-prepared carbon nitride exhibits almost 10 times higher activity than the traditional carbon nitride (calcined from melamine) in the hydrogen evolution text. As a multifunctional catalyst, the core-shell like carbon nitride also shows a superior catalytic degradation activity for RhB and p-nitrophenol.