Perspective-Outlook on Operando Photoelectron and Absorption Spectroscopy to 
Probe Catalysts at the Solid-Liquid Electrochemical Interface

Carbonio, Emilia; Velasco Vélez, Juan; Schlögl, Robert; Knop-Gericke, Axel

doi:10.1149/1945-7111/ab68d2

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Perspective-Outlook on Operando Photoelectron and Absorption Spectroscopy to Probe Catalysts at the Solid-Liquid Electrochemical Interface

MPG-Autoren

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Carbonio, Emilia
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;
Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, BESSY II, Catalysis for Energy, EM-GKAT;

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Velasco Vélez, Juan
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;
Max-Planck-Institut für Chemische Energiekonversion;

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Schlögl, Robert
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;
Max-Planck-Institut für Chemische Energiekonversion;

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Knop-Gericke, Axel
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;
Max-Planck-Institut für Chemische Energiekonversion;

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Carbonio_2020_J._Electrochem._Soc._167_054509.pdf
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Zitation

Carbonio, E., Velasco Vélez, J., Schlögl, R., & Knop-Gericke, A. (2020). Perspective-Outlook on Operando Photoelectron and Absorption Spectroscopy to Probe Catalysts at the Solid-Liquid Electrochemical Interface. Journal of the Electrochemical Society, 167(5): 054509. doi:10.1149/1945-7111/ab68d2.

Zitierlink: https://hdl.handle.net/21.11116/0000-0005-A317-9

Zusammenfassung

Operando X-ray Photoelectron and Absorption Spectroscopy (XPS and XAS) using soft (up to 2 KeV) and tender (2–10 KeV) X-rays applied to study functional materials for energy conversion has gone through great development in the last years and several approaches to different cell designs combined with instrumentation development now allow successful characterization of electrode-electrolyte interfaces under working conditions. An overview of the current state and challenges are presented along with an outlook into the direction that future development should take, which we expect would allow us to expand and complete our understanding of the liquid-solid electrochemical interfaces.