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Electron energy loss spectroscopy on freestanding perforated gold films

MPG-Autoren

Prämassing,  M.
Electron Microscopy and Analytics, Center of Advanced European Studies and Research (caesar), Max Planck Society;

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Irsen,  Stephan
Electron Microscopy and Analytics, Center of Advanced European Studies and Research (caesar), Max Planck Society;

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Zitation

Prämassing, M., Kiel, T., Irsen, S., Busch, K., & Linden, S. (2021). Electron energy loss spectroscopy on freestanding perforated gold films. Physical Review B, 103: 115403. doi:10.1103/PhysRevB.103.115403.


Zitierlink: https://hdl.handle.net/21.11116/0000-0008-4F6F-5
Zusammenfassung
We report on a combined far- and near-field study of surface plasmon polaritons on freestanding perforated gold films. The samples were fabricated by focused ion beam milling of a periodic hole array into a carbon membrane followed by thermal evaporation of gold and plasma ashing of the carbon film. Optical transmission spectra showed a series of characteristic features, which can be attributed to the excitation of surface plasmon modes via the periodic nanohole array. The corresponding near-field distributions were mapped by electron energy loss spectroscopy. In addition to the optically bright surface plasmon modes, we observed in the near-field a dark plasmon mode which is absent in the normal incidence far-field spectra. Our experimental results are in good agreement with numerical computations based on a discontinuous Galerkin time-domain method.