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Electron spin resonance study on the 4f honeycomb quantum magnet YbCl3

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Sichelschmidt,  Jörg
Jörg Sichelschmidt, Physics of Quantum Materials, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Baenitz,  M.
Michael Baenitz, Physics of Quantum Materials, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Citation

Sichelschmidt, J., Häußler, E., Vinokurova, E., Baenitz, M., & Doert, T. (2023). Electron spin resonance study on the 4f honeycomb quantum magnet YbCl3. Journal of Physics: Condensed Matter, 35(42): 425601, pp. 1-6. doi:10.1088/1361-648X/ace815.


Cite as: https://hdl.handle.net/21.11116/0000-000D-84A9-F
Abstract
The local magnetic properties of Yb3+ in the layered honeycomb material YbCl3 were investigated by electron spin resonance on single crystals. For in-plane and out-of-plane field orientations the g-factor shows a clear anisotropy ( and ), whereas the low temperature exchange coupling and the spin relaxation display a rather isotropic character. At elevated temperatures the contribution of the first excited crystal field level ( meV) dominates the spin relaxation.