Triazine-based graphitic carbon nitride thin film as a homogeneous interphase 
for lithium storage

Song, Zihan; Hou, Jing; Raguin, Emeline; Pedersen, Angus; Eren, Enis; Senokos, Evgeny; Tarakina, Nadezda V.; Giusto, Paolo; Antonietti, Markus

doi:10.1021/acsnano.3c08771

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Triazine-based graphitic carbon nitride thin film as a homogeneous interphase for lithium storage

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Song, Zihan
Paolo Giusto, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons264353

Hou, Jing
Nadezda V. Tarakina, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons264168

Raguin, Emeline
Emeline Raguin, Biomaterialien, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons285115

Eren, Enis
Paolo Giusto, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons285117

Senokos, Evgeny
Paolo Giusto, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons212917

Tarakina, Nadezda V.
Nadezda V. Tarakina, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons222676

Giusto, Paolo
Paolo Giusto, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons1057

Antonietti, Markus
Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Zitation

Song, Z., Hou, J., Raguin, E., Pedersen, A., Eren, E., Senokos, E., et al. (2024). Triazine-based graphitic carbon nitride thin film as a homogeneous interphase for lithium storage. ACS Nano, 18(3), 2066-2076. doi:10.1021/acsnano.3c08771.

Zitierlink: https://hdl.handle.net/21.11116/0000-000E-4DF9-4

Zusammenfassung

Triazine-based graphitic carbon nitride is a semiconductor material constituted of cross-linked triazine units, which differs from widely reported heptazine-based carbon nitrides. Its triazine-based structure gives rise to significantly different physical chemical properties from the latter. However, it is still a great challenge to experimentally synthesize this material. Here, we propose a synthesis strategy via vapor-metal interfacial condensation on a planar copper substrate to realize homogeneous growth of triazine-based graphitic carbon nitride films over large surfaces. The triazine-based motifs are clearly shown in transmission electron microscopy with high in-plane crystallinity. An AB-stacking arrangement of the layers is orientationlly parallel to the substrate surface. Eventually, the as-prepared films show dense electrochemical lithium deposition attributed to homogeneous charge transport within this thin film interphase, making it a promising solution for energy storage.