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  Resonances in rotationally inelastic scattering of OH(X2Π) with helium and neon

Gubbels, K., Ma, Q., Alexander, M. H., Dagdigian, P. J., Tanis, D., Groenenboom, G. C., et al. (2012). Resonances in rotationally inelastic scattering of OH(X2Π) with helium and neon. Journal of Chemical Physics, 136(14): 144308. doi:10.1063/1.3697816.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0010-1168-5 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0025-B933-F
Genre: Journal Article

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 Creators:
Gubbels, Koos1, 2, Author           
Ma, Qianli3, Author
Alexander, Millard H.4, Author
Dagdigian, Paul J.3, Author
Tanis, Dick2, Author
Groenenboom, Gerrit C.2, Author
van der Avoird, Ad2, Author
Meerakker, Bas van de2, Author           
Affiliations:
1Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
2Radboud University Nijmegen, Institute for Molecules and Materials, Heyendaalseweg 135, 6525 AJ Nijmegen, The Netherlands , ou_persistent22              
3Department of Chemistry, The Johns Hopkins University, Baltimore, Maryland 21218-2685, USA , ou_persistent22              
4Department of Chemistry and Biochemistry and Institute for Physical Science and Technology, University of Maryland, College Park, Maryland 20742-2021, USA , ou_persistent22              

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 Abstract: We present detailed calculations on resonances in rotationally and spin-orbit inelastic scattering of OH (X2Π, j = 3/2, F₁, f) radicals with He and Ne atoms. We calculate new ab initio potential energy surfaces for OH-He, and the cross sections derived from these surfaces compare well with the recent crossed beam scattering experiment of Kirste et al. [Phys. Rev. A 82, 042717 (2010)10.1103/PhysRevA.82.042717]. We identify both shape and Feshbach resonances in the integral and differential state-to-state scattering cross sections, and we discuss the prospects for experimentally observing scattering resonances using Stark decelerated beams of OH radicals.

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Language(s): eng - English
 Dates: 2012-01-162012-03-072012-04-112012-04-14
 Publication Status: Issued
 Pages: 13
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1063/1.3697816
 Degree: -

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Title: Journal of Chemical Physics
  Other : J. Chem. Phys.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Institute of Physics
Pages: - Volume / Issue: 136 (14) Sequence Number: 144308 Start / End Page: - Identifier: ISSN: 0021-9606
CoNE: https://pure.mpg.de/cone/journals/resource/954922836226