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  A sustainable synthesis alternative for IL-derived N-doped carbons : bio-based-imidazolium compounds

Yang, S. J., Rothe, R., Kirchhecker, S., Esposito, D., Antonietti, M., Gojzewski, H., et al. (2015). A sustainable synthesis alternative for IL-derived N-doped carbons: bio-based-imidazolium compounds. Carbon, 94, 641-645. doi:10.1016/j.carbon.2015.07.034.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0027-C37A-9 Version Permalink: https://hdl.handle.net/21.11116/0000-000B-40D5-C
Genre: Journal Article

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 Creators:
Yang, Seung Jae1, Author           
Rothe, Regina1, Author           
Kirchhecker, Sarah2, Author           
Esposito, Davide2, Author           
Antonietti, Markus3, Author           
Gojzewski, Hubert4, Author           
Fechler, Nina5, Author           
Affiliations:
1Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863288              
2Davide Esposito, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863315              
3Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              
4Hans Riegler, Grenzflächen, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863311              
5Tim Fellinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863322              

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 Abstract: Herein we report a facile and scalable synthesis of highly nitrogen-doped porous carbon materials with tunable morphology. Bio-based imidazolium derivatives made from natural amino acids and dioxo-derivatives are employed as precursors, exhibiting an analogous behavior during carbonization to classical ionic liquids. Utilization of systematically controlled salt templating methods yields nitrogen-doped carbon materials with high surface areas of up to 2650 m2 g-1 and morphology-engineered structures such as monolithic or highly extended, sheet-like carbons. We believe that the presented approach represents an alternative and sustainable platform towards the rational design of carbon materials possessing controlled nanoporosity and functionality.

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 Dates: 2015-07-092015
 Publication Status: Issued
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 Identifiers: URI: http://www.sciencedirect.com/science/article/pii/S0008622315300579
DOI: 10.1016/j.carbon.2015.07.034
DOI: 10.1016/j.carbon.2016.07.029
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Title: Carbon
Source Genre: Journal
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Publ. Info: Amsterdam : Elsevier
Pages: - Volume / Issue: 94 Sequence Number: - Start / End Page: 641 - 645 Identifier: ISSN: 0008-6223