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  Strongly driven quantum pendulum of the carbonyl sulfide molecule

Trippel, S., Mullins, T., Müller, N. L. M., Kienitz, J. S., Omiste, J. J., Stapelfeldt, H., et al. (2014). Strongly driven quantum pendulum of the carbonyl sulfide molecule. Physical Review A, 89(5): 051401(R). doi:10.1103/PhysRevA.89.051401.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002A-E909-3 Version Permalink: https://hdl.handle.net/21.11116/0000-0007-0EA9-C
Genre: Journal Article

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PhysRevA.89.051401.pdf (Publisher version), 2MB
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http://dx.doi.org/10.1103/PhysRevA.89.051401 (Publisher version)
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https://arxiv.org/abs/1401.6897 (Preprint)
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 Creators:
Trippel, Sebastian1, Author
Mullins, Terry1, Author
Müller, Nele L. M.1, 2, Author           
Kienitz, Jens S.1, 3, Author
Omiste, Juan J.4, Author
Stapelfeldt, Henrik5, 6, Author
González-Férez, Rosario3, 4, Author
Küpper, Jochen1, 3, 7, Author
Affiliations:
1Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany, ou_persistent22              
2International Max Planck Research School for Ultrafast Imaging & Structural Dynamics (IMPRS-UFAST), Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266714              
3The Hamburg Center for Ultrafast Imaging, University of Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany, ou_persistent22              
4Instituto Carlos I de Física Teórica y Computacional and Departamento de Física Atómica, Molecular y Nuclear, Universidad de Granada, 18071 Granada, Spain, ou_persistent22              
5Department of Chemistry, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
6Interdisciplinary Nanoscience Center (iNANO), Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
7Department of Physics, University of Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany, ou_persistent22              

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Free keywords: PACS numbers: 33.80.−b, 37.10.Vz, 37.20.+j
 Abstract: We demonstrate and analyze a strongly driven quantum pendulum in the angular motion of state-selected and laser-aligned carbonyl sulfide molecules. Raman couplings during the rising edge of a 50-ps laser pulse create a wave packet of pendular states, which propagates in the confining potential formed by the polarizability interaction between the molecule and the laser field. This wave-packet dynamics manifests itself as pronounced oscillations in the degree of alignment with a laser-intensity-dependent period.

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Language(s): eng - English
 Dates: 2014-01-272014-05-052014-05
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevA.89.051401
arXiv: 1401.6897
 Degree: -

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Title: Physical Review A
  Other : Phys. Rev. A
  Other : Physical Review A: Atomic, Molecular, and Optical Physics
Source Genre: Journal
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Publ. Info: New York, NY : American Physical Society
Pages: - Volume / Issue: 89 (5) Sequence Number: 051401(R) Start / End Page: - Identifier: ISSN: 1050-2947
CoNE: https://pure.mpg.de/cone/journals/resource/954925225012_2