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  X-ray photoelectron spectroscopy and near-edge X-ray absorption fine structure study of water adsorption on pyridine-terminated thiolate self-assembled monolayers

Zubavichus, Y., Zharnikov, M., Yang, Y., Fuchs, O., Umbach, E., Heske, C., et al. (2004). X-ray photoelectron spectroscopy and near-edge X-ray absorption fine structure study of water adsorption on pyridine-terminated thiolate self-assembled monolayers. Langmuir, 20(25), 11022-11029. doi:10.1021/la047980b.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0001-ADA2-5 Version Permalink: https://hdl.handle.net/21.11116/0000-0001-ADA3-4
Genre: Journal Article

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Langmuir_20_2004_11022.pdf (Any fulltext), 198KB
 
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https://pubs.acs.org/doi/pdf/10.1021/la047980b (Any fulltext)
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 Creators:
Zubavichus, Yan, Author
Zharnikov, Michael, Author
Yang, Yongjie, Author
Fuchs, Oliver, Author
Umbach, Eberhard, Author
Heske, Clemens, Author
Ulman, Abraham, Author
Grunze, Michael1, Author           
Affiliations:
1Cellular Biophysics, Max Planck Institute for Medical Research, Max Planck Society, ou_2364731              

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 Abstract: Adsorption of water on self-assembled monolayers (SAMs) of 4-(4-mercaptophenyl)pyridine on gold at low temperatures under ultrahigh vacuum conditions is studied by synchrotron radiation X-ray photoelectron and absorption spectroscopy. Water adsorption induces a strong modification of the chemical state of the pyridine N atoms at the SAM/ice interface, indicative for strong H bonding and partial proton transfer between water molecules and pyridine moieties. Additionally, the initial molecular orientation within the SAM is changed upon formation of an adsorbed water multilayer.

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Language(s): eng - English
 Dates: 2004-08-122004-09-202004-11-06
 Publication Status: Issued
 Pages: 8
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/la047980b
URI: https://www.ncbi.nlm.nih.gov/pubmed/15568854
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Title: Langmuir
Source Genre: Journal
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Publ. Info: Columbus, OH : American Chemical Society
Pages: - Volume / Issue: 20 (25) Sequence Number: - Start / End Page: 11022 - 11029 Identifier: ISSN: 0743-7463
CoNE: https://pure.mpg.de/cone/journals/resource/954925541194