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  Characterisation of three terpene synthases for β-barbatene, β-araneosene and nephthenol from social amoebae

Rinkel, J., Köllner, T. G., Chen, F., & Dickschat, J. S. (2019). Characterisation of three terpene synthases for β-barbatene, β-araneosene and nephthenol from social amoebae. Chemical Communications, 55(88), 13255-13258. doi:10.1039/c9cc07681f.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0004-E15E-5 Version Permalink: https://hdl.handle.net/21.11116/0000-0009-30CF-8
Genre: Journal Article

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GER581.pdf (Publisher version), 2MB
 
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GER581s1.pdf (Supplementary material), 14MB
 
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Rinkel, J., Author
Köllner, Tobias G.1, Author           
Chen, F., Author
Dickschat, J. S., Author
Affiliations:
1Department of Biochemistry, Prof. J. Gershenzon, MPI for Chemical Ecology, Max Planck Society, ou_421893              

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 Abstract: The products of three terpene synthases from two social amoebae, Dictyostelium discoideum and Dictyostelium purpureum, were identified, showing sesquiterpene synthase activity for one and diterpene synthase activity for the other two enzymes. Site-directed mutagenesis experiments revealed the importance of a newly identfied highly conserved residue for catalytic activity. For one of the enzyme products, β-araneosene, a bromonium ion induced transannular cyclisation was investigated, yielding the first brominated derivatives of this diterpene.

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 Dates: 2019-10-112019-10-172019-11
 Publication Status: Issued
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 Rev. Type: -
 Identifiers: Other: GER581
DOI: 10.1039/c9cc07681f
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Title: Chemical Communications
  Other : Chem. Commun.
Source Genre: Journal
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Publ. Info: Cambridge, UK : Royal Society of Chemistry
Pages: - Volume / Issue: 55 (88) Sequence Number: - Start / End Page: 13255 - 13258 Identifier: ISSN: 1359-7345
CoNE: https://pure.mpg.de/cone/journals/resource/954928495413