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  Angstrom-Resolved Interfacial Structure in Buried Organic-Inorganic Junctions

Schwartz, C. P., Raj, S. L., Jamnuch, S., Hull, C. J., Miotti, P., Lam, R. K., et al. (2021). Angstrom-Resolved Interfacial Structure in Buried Organic-Inorganic Junctions. Physical Review Letters, 127(9): 096801. doi:10.1103/PhysRevLett.127.096801.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0006-611B-F Version Permalink: https://hdl.handle.net/21.11116/0000-0009-22F9-8
Genre: Journal Article

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 Creators:
Schwartz, Craig P.1, Author
Raj, Sumana L.2, Author
Jamnuch, Sasawat3, Author
Hull, Chris J.1, 2, Author
Miotti, Paolo4, 5, Author
Lam, Royce K.1, 2, Author
Nordlund, Dennis6, Author
Uzundal, Can B.2, Author
Pemmaraju, Chaitanya Das7, Author
Mincigrucci, Riccardo8, Author
Foglia, Laura8, Author
Simoncig, Alberto8, Author
Coreno, Marcello9, 10, Author
Masciovecchio, Claudio8, Author
Giannessi, Luca8, 10, Author
Poletto, Luca4, Author
Principi, Emiliano8, Author
Zürch, Michael2, 11, 12, 13, Author           
Pascal, Tod A.3, 14, 15, Author
Drisdell, Walter S.1, 16, Author
Saykally, Richard J.1, 2, Author more..
Affiliations:
1Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA, ou_persistent22              
2Department of Chemistry, University of California, Berkeley, California 94720, USA, ou_persistent22              
3ATLAS Materials Science Laboratory, Department of NanoEngineering and Chemical Engineering, University of California, San Diego, La Jolla, California 92023, USA, ou_persistent22              
4Institute of Photonics and Nanotechnologies, National Research Council of Italy, via Trasea 7, I-35131 Padova, Italy, ou_persistent22              
5Department of Information Engineering, University of Padova, via Gradenigo 6/B, I-35131 Padova, Italy, ou_persistent22              
6Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA, ou_persistent22              
7Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA, ou_persistent22              
8Elettra-Sincrotrone Trieste S.C.p.A., Strada Statale 14—km 163.5, 34149 Trieste, Italy, ou_persistent22              
9ISM-CNR, Istituto di Struttura della Materia, LD2 Unit, 34149 Trieste, Italy, ou_persistent22              
10Istituto Nazionale di Fisica Nucleare, Laboratori Nazionali di Frascati, Via E. Fermi 54, 00044 Frascati, Italy, ou_persistent22              
11Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
12Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA, ou_persistent22              
13Institute for Optics and Quantum Electronics, Abbe Center of Photonics, University of Jena, 07745 Jena, Germany, ou_persistent22              
14Materials Science and Engineering, University of California San Diego, La Jolla, California 92023, USA, ou_persistent22              
15Sustainable Power and Energy Center, University of California San Diego, La Jolla, California 92023, USA, ou_persistent22              
16Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA, ou_persistent22              

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Free keywords: Condensed Matter, Materials Science, cond-mat.mtrl-sci
 Abstract: Charge transport processes at interfaces play a crucial role in many processes. Here, the first soft x-ray second harmonic generation (SXR SHG) interfacial spectrum of a buried interface (boron–Parylene N) is reported. SXR SHG shows distinct spectral features that are not observed in x-ray absorption spectra, demonstrating its extraordinary interfacial sensitivity. Comparison to electronic structure calculations indicates a boron-organic separation distance of 1.9 Å, with changes of less than 1 Å resulting in easily detectable SXR SHG spectral shifts (ca. hundreds of milli-electron volts).

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Language(s): eng - English
 Dates: 2020-05-042021-02-242021-07-022021-08-242021-08-27
 Publication Status: Issued
 Pages: 6
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: arXiv: 2005.01905
DOI: 10.1103/PhysRevLett.127.096801
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: 6 Volume / Issue: 127 (9) Sequence Number: 096801 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1