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  Selective oxidation of alcohols using carbon nitride photocatalysts

Savateev, A. (2023). Selective oxidation of alcohols using carbon nitride photocatalysts. In X. Wang, M. Anpo, & X. Fu (Eds.), UV-visible photocatalysis for clean energy production and pollution remediation (pp. 27-40). Weinheim: Wiley-VCH GmbH. doi:10.1002/9783527837991.ch3.

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Item Permalink: https://hdl.handle.net/21.11116/0000-000D-9288-4 Version Permalink: https://hdl.handle.net/21.11116/0000-000D-9299-1
Genre: Book Chapter

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Chapter.pdf (Publisher version), 506KB
 
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 Creators:
Savateev, Aleksandr1, Author                 
Affiliations:
1Aleksandr Savateev, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2421702              

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Free keywords: heterogeneous photocatalysis; carbon nitride; visible light; superoxide radical; oxidation of alcohols; elemental sulfur; flow photocatalysis; semiconductor photo-charging; hydrogen peroxide
 Abstract: The oxidation of alcohols mediated by semiconductor materials was one of the first organic photocatalytic reactions reported as early as the 1960s. Today, it is one of the most studied reactions in photocatalysis. The chapter summarizes a reaction mechanism of alcohol oxidation with O 2 mediated by carbon nitride photocatalysts. Selectivity toward carbonyl compounds and strategies adopted in carbon nitride research to improve selectivity are discussed. These strategies include performing the reaction in flow, the substitution of O 2 with other oxidants, such as S 8 , and employing hydrogen-evolving cocatalysts or photo-chargeable carbon nitrides to enable selective dehydrogenation of primary alcohols.

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Language(s): eng - English
 Dates: 2023-02-172023
 Publication Status: Issued
 Pages: -
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 Table of Contents: -
 Rev. Type: -
 Identifiers: DOI: 10.1002/9783527837991.ch3
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Title: UV-visible photocatalysis for clean energy production and pollution remediation
Source Genre: Book
 Creator(s):
Wang, Xinchen, Editor
Anpo, Masakazu, Editor
Fu, Xianzhi, Editor
Affiliations:
-
Publ. Info: Weinheim : Wiley-VCH GmbH
Pages: 340 Seiten Volume / Issue: - Sequence Number: - Start / End Page: 27 - 40 Identifier: ISBN: 9783527350506