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  Dissolved Carbon Controls the Initial Stages of Nanocarbon Growth

Rinaldi, A., Tessonnier, J.-P., Schuster, M. E., Blume, R., Girgsdies, F., Zhang, Q., et al. (2011). Dissolved Carbon Controls the Initial Stages of Nanocarbon Growth. Angewandte Chemie International Edition, 50(14), 3313-3317. doi:10.1002/anie.201006639.

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 Creators:
Rinaldi, Ali1, Author              
Tessonnier, Jean-Philippe1, Author              
Schuster, Manfred Erwin1, Author              
Blume, Raoul1, Author              
Girgsdies, Frank1, Author              
Zhang, Qiang1, Author              
Jacob, Timo2, Author
Abd Hamid, Sharifah Bee3, Author
Su, Dang Sheng1, 4, Author              
Schlögl, Robert1, Author              
Affiliations:
1Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              
2Universität Ulm, Albert-Einstein-Allee 47, 89081 Ulm (Germany, ou_persistent22              
3Combinatorial Technology and Catalyst Research Centre (COMBICAT, ou_persistent22              
4Shenyang National Laboratory for Materials Science Institute of Metal Research, Chinese Academy of Science, 72 Wenhua Road, Shenyang 110016 (China), ou_persistent22              

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Free keywords: carbon nanotubes; dissolved carbon; nanoparticle catalysts; nickel; supported catalysts
 Abstract: Sneaked in: Carbon atoms from defective supports are incorporated in nickel nanoparticles at relatively low temperatures (for example in a Ni(100) surface; Ni brown, C black) The dissolved carbon not only modifies the electronic properties of the metal but it also leads to a reconstruction of the nanoparticles. These findings may explain many of the differences in catalytic activity observed when supporting metals on carbon.

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Language(s): eng - English
 Dates: 2011-02-242011-03-28
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.201006639
 Degree: -

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Title: Angewandte Chemie International Edition
Source Genre: Journal
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Publ. Info: Weinheim/Bergstr. : Verlag Chemie
Pages: - Volume / Issue: 50 (14) Sequence Number: - Start / End Page: 3313 - 3317 Identifier: ISSN: 0570-0833
CoNE: https://pure.mpg.de/cone/journals/resource/110984073528720