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Technical Note: Atmospheric CO2 inversions on the mesoscale using data-driven prior uncertainties: methodology and system evaluation

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Kountouris,  Panagiotis
IMPRS International Max Planck Research School for Global Biogeochemical Cycles, Max Planck Institute for Biogeochemistry, Max Planck Society;

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Gerbig,  Christoph
Airborne Trace Gas Measurements and Mesoscale Modelling, Dr. habil. C. Gerbig, Department Biogeochemical Systems, Prof. M. Heimann, Max Planck Institute for Biogeochemistry, Max Planck Society;

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Rödenbeck,  Christian
Inverse Data-driven Estimation, Dr. C. Rödenbeck, Department Biogeochemical Systems, Prof. M. Heimann, Max Planck Institute for Biogeochemistry, Max Planck Society;

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Karstens,  Ute
Regional Scale Modelling of Atmospheric Trace Gases, Dr. U. Karstens, Department Biogeochemical Systems, Prof. M. Heimann, Max Planck Institute for Biogeochemistry, Max Planck Society;

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Heimann,  Martin
Department Biogeochemical Systems, Prof. M. Heimann, Max Planck Institute for Biogeochemistry, Max Planck Society;

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Citation

Kountouris, P., Gerbig, C., Rödenbeck, C., Karstens, U., Koch, T. F., & Heimann, M. (2018). Technical Note: Atmospheric CO2 inversions on the mesoscale using data-driven prior uncertainties: methodology and system evaluation. Atmospheric Chemistry and Physics, 18(4), 3027-3045. doi:10.5194/acp-18-3027-2018.


Cite as: https://hdl.handle.net/11858/00-001M-0000-002E-2445-D
Abstract
Atmospheric inversions are widely used in the optimization of surface carbon fluxes on a regional scale using information from atmospheric CO2 dry mole fractions. In many studies the prior flux uncertainty applied to the inversion schemes does not directly reflect the true flux uncertainties but is used to regularize the inverse problem. Here, we aim to implement an inversion scheme using the Jena inversion system and applying a prior flux error structure derived from a model–data residual analysis using high spatial and temporal resolution over a full year period in the European domain. We analyzed the performance of the inversion system with a synthetic experiment, in which the flux constraint is derived following the same residual analysis but applied to the model–model mismatch. The synthetic study showed a quite good agreement between posterior and “true” fluxes on European, country, annual and monthly scales. Posterior monthly and country-aggregated fluxes improved their correlation coefficient with the “known truth” by 7% compared to the prior estimates when compared to the reference, with a mean correlation of 0.92. The ratio of the SD between the posterior and reference and between the prior and reference was also reduced by 33% with a mean value of 1.15. We identified temporal and spatial scales on which the inversion system maximizes the derived information; monthly temporal scales at around 200 km spatial resolution seem to maximize the information gain.