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Journal Article

Hydroamination of Aromatic Alkynes to Imines Catalyzed by Pd(II)-Anthraphos Complexes

MPS-Authors
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Erken,  Christina
Research Department Leitner, Max Planck Institute for Chemical Energy Conversion, Max Planck Society;

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Hindemith,  Carsten
Research Department Schlögl, Max Planck Institute for Chemical Energy Conversion, Max Planck Society;

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Weyhermüller,  Thomas
Research Department DeBeer, Max Planck Institute for Chemical Energy Conversion, Max Planck Society;

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Werlé,  Christophe
Research Department Schlögl, Max Planck Institute for Chemical Energy Conversion, Max Planck Society;

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Leitner,  Walter
Research Department Leitner, Max Planck Institute for Chemical Energy Conversion, Max Planck Society;
Institut für Technische Chemie und Makromolekulare Chemie, Rheinisch‐Westfälische Technische Hochschule Aachen, Worringer Weg 1, 52074 Aachen, Germany;

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Citation

Erken, C., Hindemith, C., Weyhermüller, T., Hölscher, M., Werlé, C., & Leitner, W. (2020). Hydroamination of Aromatic Alkynes to Imines Catalyzed by Pd(II)-Anthraphos Complexes. ACS Omega, 5(15), 8912-8918. doi:10.1021/acsomega.0c00562.


Cite as: https://hdl.handle.net/21.11116/0000-0007-A49D-F
Abstract
Herein, we report the synthesis, characterization, and catalytic performance of cationic Pd(II)-Anthraphos complexes in the intermolecular hydroamination of aromatic alkynes with aromatic amines. The reaction proceeds with 0.18 mol % of catalyst loading, at 90 degrees C for 4 h under neat conditions. Good to excellent yields could be obtained for a broad range of amines and alkynes.