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C2NxO1-x framework carbons with defined microporosity and Co-doped functional pores

MPG-Autoren
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Tian,  Zhihong
Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Fechler,  Nina
Nina Fechler, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Oschatz,  Martin
Martin Oschatz, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Heil,  Tobias
Nadezda V. Tarakina, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Antonietti,  Markus
Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Zitation

Tian, Z., Fechler, N., Oschatz, M., Heil, T., Schmidt, J., Yuan, S., et al. (2018). C2NxO1-x framework carbons with defined microporosity and Co-doped functional pores. Journal of Materials Chemistry A, 6(39), 19013-19019. doi:10.1039/C8TA03213K.


Zitierlink: https://hdl.handle.net/21.11116/0000-0002-18F7-D
Zusammenfassung
Gallic acid and urea are used to produce C2NO materials with rather dined micropores via direct condensation and ring closure. The materials show a unique heterocycle containing carbonaceous structure and features an unusually high content of heteroatoms (nitrogen, oxygen) lining inside the pores, meanwhile having high specific surface area. The multifunctional carbon materials demonstrate good performance for selective CO2 capture resulting from the adjustable porosity and polarizability. In view of the simplicity of the salt flux synthetic method and the advantage of the available sustainable starting synthons, the C2NO framework has potential for use in diverse practical applications.